Publication date: 21st July 2025
Individual quantum dots (QDs) serve as inherent sources for quantum states of light such as single photons and entangled photon pairs. Ideally, under cryogenic conditions, their radiation is fully coherent – maintaining a constat phase relation throughout the emission lifetime. Often, however, the interaction of excited electrons with the lattice limits the coherence lifetime to the picosecond timescale. Experimentally, such a timescale necessitates the use of pump-probe measurements with ultrashort laser pulses. While the generation of short pulses is hardly a novelty, applying them to the sensitive spectroscopy of single nano objects is a highly challenging task. Here, we present the first transient-transmission experiments directly measuring the coherent dynamics of excitons in an individual epitaxial CdSe QD.
Using a highly stable femtosecond Er:fiber laser source, we generate the pump and probe beams that are focused through a high-numerical-aperture objective within an optical cryostat (T=1.6 K). Exciting well above the lowest-energy transition (
The unprecedented capability of our setup to expose the full energy landscape of a single confined exciton and its dynamics following excitation promises to bring to light new physics in the realm of nano and quantum optics.