Publication date: 8th July 2026
Indistinguishable single photons are a fundamental resource for photonic quantum technologies, but their generation from scalable colloidal quantum emitters remains hindered by decoherence, spectral diffusion and slow radiative dynamics. Here we demonstrate near-transform-limited single-photon emission from individual lead-halide perovskite nanorods exhibiting strongly linearly polarized single-line emission and exceptionally short radiative lifetimes. The elongated nanorod geometry simultaneously enables coherent exciton delocalization in the weak confinement regime and suppresses dielectric depolarization for the longitudinal transition, concentrating the oscillator strength into a single bright dipole. Together, these effects give rise to giant oscillator strength and single-exciton superradiance, producing exceptionally short radiative lifetimes that reduce the relative impact of dephasing processes and enable optical coherence approaching the transform limit, as confirmed by Fourier correlation spectroscopy. Two-photon quantum interference measurements based on the Hong–Ou–Mandel effect reveal highly indistinguishable photon emission from individual nanorods. Statistical analysis performed over 26 individual nanorods yields average raw and corrected visibilities of ~40% and ~50%, respectively. For nanorods on which the emission spectrum, lifetime, optical coherent time, photon statistics and Hong–Ou–Mandel interference could be simultaneously monitored throughout the measurement, corrected photon indistinguishability visibilities reach up to 80%. Ultrafast streak-camera measurements identify hot-carrier cooling occurring on a few-picosecond timescale as a residual source of temporal jitter introduced by non-resonant excitation and limiting two-photon interference. Taking this contribution into account indicates that resonantly excited nanorods could approach near-unity photon indistinguishability.
